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Lovely article, Tim, just as last year.
Though I may have to use WebKit animations and transitions on live sites, I’ve found that using it during the design process is a great way to quickly test out user interface experience ideas. If it’s necessary for functionality, I try to replicate it as well as possible with jQuery before going live. These things belong in CSS, though (IMHO), and I sure hope that this is what the future will look like.